What is the finding
Researchers discovered unusual electronic behavior at the interfaces of special oxides, where electrons move in surprising patterns that break long-standing theories of quantum physics. According to conventional theory, these oscillations should be periodic in the inverse magnetic field. However, in complex oxide interfaces such as LaAlO3/SrTiO3 and LaAlO3/KTaO3, the oscillation frequency increases progressively with increasing magnetic field strength, indicating the presence of nontrivial electronic states.
Why is this important?
Despite being made from insulating materials, certain oxide interfaces can conduct electricity and even show superconductivity and magnetism—features useful for future memory and quantum technologies. To understand why and how this works, researchers studied the behavior of electrons at three different oxide interfaces using high magnetic fields. They observed unconventional quantum oscillations, showing that electrons follow unique energy pathways that mix two different types of motion. Our experimental findings and versatile theoretical model also hold promise for comprehending similar observations in other materials with strong spin-orbit coupling, including Dirac and Weyl semimetals.
Who did the research?
K. Rubi1, D. R. Candido2, M. Dumen3, S. Zeng4, E. Ammerlaan5, F. Bangma5, M. Chan1, M. Goiran6, A. Ariando4, S. Chakraverty3, W. Escoffier6, U. Zeitler5, N.Harrison1
1National MagLab, Los Alamos National laboratory; 2University of Iowa; 3Institute of Nano Science and Technology, India; 4National University of Singapore, Singapore; 5HFML-EMFL, Radboud University Netherlands; 6LNCMI-EMFL, Toulouse France.
Why did they need the MagLab?
Because electrons do not move very quickly in these oxide interfaces (moderate electron mobility), extremely high magnetic fields—up to 60 T—were essential to resolve the quantum oscillations and see the quantum behavior. Higher magnetic fields are needed to observe a sufficient number of oscillations (typically 8–10) to reliably identify these materials’ unconventional nature.
Details for scientists
- View or download the expert-level Science Highlight, Unconventional quantum oscillations in complex oxide interfaces
- Read the full-length publication, Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces, in Physical Review Research
Funding
This research was funded by the following grants: G.S. Boebinger (NSF DMR-1644779); Neil Harrison (DoE “Science of 100 Tesla”)
For more information, contact Neil Harrison.